At a very young age, Mary-Charles Jones' family quickly noticed that she had an ability to captivate strangers with her outgoing personality. And at the ripe young age of 4, her family decided to bring her to an open call held by local agent Joy Pervis where she was immediately signed for both local representation and national representation through Osbrink.

Quickly Mary-Charles began booking in print, local, regional, and national commercials and television and film roles were soon to follow. Her first job in that capacity was a recurring role as "Caitlin Rowan" in the ABC drama October Road and it began to waterfall from there. Mary-Charles' ability to handle emotional story lines allowed for her to be cast in a heart wrenching episode of ABC's hit series Grey's Anatomy, she had the honor of working with Kevin Spacey in the film Father of Invention, and she was cast to play a young Miley Cyrus in a recurring capacity on Hannah Montana. More recently Mary-Charles was cast in a guest starring role opposite Zooey Deschanel in New Girl.

Mary-Charles had the opportunity to work with her sister Maggie Elizabeth Jones for the first time playing sisters in Paramount's remake of Footloose. They would get to do this again a few years later in Universal's Identity Thief opposite Jason Bateman and Melissa McCarthy.

Mary-Charles can also be seen as the lead role of Isabella in Walden Media's film Dear Dumb Diary, which is based on the Scholastic's popular children's book series by the same name.

Mary-Charles Jones was born on December 28, 2001 in Seattle, Washington. In Late 2002 Mary-Charles family relocated to Atlanta, Georgia where they still reside