Papa Smurf / Azrael / Dreamy Smurf / Barber Smurf / Rogue / Sickly Smurf / Captain Cookie / Cohort / Dreamy / Fallon / Peasant (255 episodes, 1981-1989)
Brainy Smurf / King Smurf (248 episodes, 1981-1989)
Smurfette (237 episodes, 1981-1989)
Handy Smurf / Grouchy Smurf / Lazy Smurf / Johan / El Gargo / Garganzole / Gargapuri / Gargovich / Van Garg (236 episodes, 1981-1989)
Hefty Smurf / Poet Smurf / Peewit / Wild Smurf / Clockwork Smurf / Mouse Master / Nemesis / Commentator / Dr. Charlatan / Hermit / The Prince (233 episodes, 1981-1989)
Clumsy Smurf / Painter Smurf / Don Smurfo (227 episodes, 1981-1989)
Greedy Smurf / Harmony Smurf / Woody (225 episodes, 1981-1989)
Vanity Smurf / Father Time / Wislow (162 episodes, 1981-1989)
Gargamel / Baby Smurf / Flighty Smurf (159 episodes, 1981-1988)
Jokey Smurf / Mother Nature / Mummy / Mrs. Sourberry / Sea Witch (155 episodes, 1981-1989)
Sassette Smurfling / Baby Smurf (110 episodes, 1984-1989)
Farmer Smurf / Miner Smurf / Scaredy Smurf / Additional voices / McKilty (97 episodes, 1981-1989)
Snappy Smurfling / Snappy Smurf (92 episodes, 1984-1989)
Natural 'Nat' Smurfling / Grogg (75 episodes, 1984-1989)
Slouchy Smurfling (71 episodes, 1984-1989)
Tailor Smurf / Tracker Smurf (64 episodes, 1982-1988)
Grandpa Smurf (63 episodes, 1984-1989)
Scruple / Additional Voices / Architect Smurf / Scrupsis (53 episodes, 1984-1989)
Bigmouth / Additional Voices (28 episodes, 1981-1989)
Smoogle / Additional Voices / Brenda / Laura (26 episodes, 1982-1989)
Chlorhydris / Dame Barbara / Additional Voices (26 episodes, 1982-1989)
Homnibus / Additional Voices (24 episodes, 1982-1989)
Hogatha / Additional Voices / Esmeralda Fortune (20 episodes, 1981-1989)
Balthazar / Additional Voices (18 episodes, 1982-1989)
King Bullrush / Additional Voices / Julius Geezer (17 episodes, 1981-1989)
Sludge / Additional Voices / Gizmo Boggs / Mr. Knott (17 episodes, 1982-1987)
Slime / Selwyn Quarrel / Additional Voices / Cousin McDougall / Wizard Anton (15 episodes, 1984-1989)
Additional Voices / Mummy / Antipasto / Babbling Brooke / Esmeralda Fortune / Gowagga Puppet / Matilda / Mrs. Sourberry / Priscilla / Queen Felicity / Rose (14 episodes, 1981-1989)
Nanny Smurf / Pansy / Additional Voices (14 episodes, 1984-1989)
Good King (13 episodes, 1982-1983)
Tracker Smurf / Additional Voices / Wizard Cheswick (13 episodes, 1982-1989)
Devil Smurf / Additional Voices / Custodian of Avalon (13 episodes, 1983-1988)
Natural Smurf / Additional Voices (11 episodes, 1983-1985)
King Gerard / Additional Voices (11 episodes, 1981-1987)
Princess Sabina / Additional Voices / Francis (10 episodes, 1982-1989)
Angel Smurf / Additional Voices (10 episodes, 1984-1988)
Weepy Smurf / Andrea / Flowerbell (9 episodes, 1982-1987)
Additional Voices / Boggie / Captain Wartmore / Federico Fettucini / Ivan Ivanovich / Marco Smurf / The Prince / Young Gargamel (9 episodes, 1985-1989)
Additional Voices / Malakov / Imp / Malchior (7 episodes, 1981-1987)
Bignose / Additional Voices (7 episodes, 1984-1986)
Sloppy Smurf (6 episodes, 1982)
Tuffy Smurf / Additional Voices (6 episodes, 1984-1989)
Timber Smurf / Additional Voices (6 episodes, 1985-1987)
Additional Voices / Blue Eyes' Mother / Simon / Sylvia (6 episodes, 1982-1989)
Additional Voices / Gluttonous / Great Book of Spells / Marsh Monster / Sir Lancealout / Zues (6 episodes, 1981-1989)
Gourdy / Additional Voices / Mr. Poppery (5 episodes, 1981-1986)
Elderberry / Additional Voices (5 episodes, 1983-1984)
Additional Voices / Wooly Smurf (5 episodes, 1985-1989)
Additional Voices / Pepper Pirate (5 episodes, 1982-1989)
Ali Baby / Additional Voices / Adella (4 episodes, 1987-1989)
Additional Voices / Morlock (4 episodes, 1982-1986)
Additional Voices / Tebuli the Genie (4 episodes, 1984-1989)
Additional Voices (4 episodes, 1982-1989)
Additional Voices / Pushover Smurf (4 episodes, 1982-1988)
Additional Voices (4 episodes, 1981-1987)
Additional Voices (4 episodes, 1981-1984)
Acorn (3 episodes, 1984)
Denisa / Additional Voices (3 episodes, 1988)
Additional Voices / Evelyn / Morgan Lafay (3 episodes, 1987-1989)
Additional Voices / Petaluma (3 episodes, 1986-1989)
Additional Voices (3 episodes, 1982-1988)
Additional Voices (3 episodes, 1982-1987)
Additional Voices (3 episodes, 1982-1984)
Additional Voices (3 episodes, 1983-1988)
Additional Voices (3 episodes, 1984-1987)
Additional Voices / The Sultan of Sweets (2 episodes, 1989)
Additional Voices (2 episodes, 1986-1989)
Additional Voices / Grako (2 episodes, 1982)
Additional Voices (2 episodes, 1987-1989)
Additional Voices / Nosey Smurf (2 episodes, 1982)
Additional Voices (2 episodes, 1984-1989)
Additional Voices / The Gamemaster (2 episodes, 1985)
Additional Voices / Merlin (1 episode, 1989)
Additional Voices / Blue Eyes (1 episode, 1984)
Additional Voices / Madame Hildegarde (2 episodes, 1987)
Additional Voices / Lady Luck (2 episodes, 1987)
Additional Voices / Teacher (2 episodes, 1984-1986)
Additional Voices (2 episodes, 1988-1989)
Additional Voices (2 episodes, 1982-1989)
Additional Voices (2 episodes, 1981-1986)
Additional Voices (2 episodes, 1981-1982)
Additional Voices (2 episodes, 1982-1988)
Additional Voices (2 episodes, 1983-1984)
Additional Voices (2 episodes, 1984-1986)
Additional Voices (2 episodes, 1984-1985)
Additional Voices (2 episodes, 1985-1987)
Additional Voices (2 episodes, 1985-1986)
Additional Voices (2 episodes, 1986-1987)
Additional Voices (2 episodes, 1987-1988)
Cupid (1 episode, 1986)
Brenda (1 episode, 1983)
Additional Voices (1 episode, 1989)
The ambassador (1 episode, 1983)
Additional Voices (1 episode, 1982)
(1 episode, 1983)
Additional Voices (1 episode, 1984)
Additional Voices (1 episode, 1986)
Rick / Warden (1 episode, 1986)
Drusilla (1 episode, 1987)
Additional Voices (1 episode, 1987)
Additional Voices (1 episode, 1988)
Additional Voices (uncredited) (1 episode, 1984)
Additional Voices (uncredited) (1 episode, 1987)
Additional Voices (uncredited) (1 episode, 1988)